I'd say (if I can chip in), that if you got those three covered ('Moondawn' being his perhaps weakest offering of the 70's..). Then I'd go first for 'Irrlicht', 'Cyborg' and 'Picture Music' (+ all the Cosmic Jokers/Couriers collaborations, Sand etc..) and then take it from there.
They aren't exactly overflowing out of the bins anymore, but can still (at least for now..) found in rather moderate prices when compared to other Krautrock in general. Don't know about Canada though...
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